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袁自冰
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袁自冰,男,博士后,教授,2002年獲北京大學化學學士,2006年獲香港科技大學大氣環境科學博士學位,畢業后留校工作,歷任博士后,副研究員,研究助理教授,同時已在國際知名雜志(SCI收錄)發表論文三十余篇,其中第一作者或通訊作者十余篇,2015年以來主持多項國家以及省部級重點項目,2017年3月份入選“大氣污染成因與控制技術研究”重點專項視頻評審專家,經濟快速發展地區區域空氣質量改善國際系列學術會議重要組織者之一。

人物經歷

1998.9 – 2002.7 北京大學理學學士(化學) 2002.9 – 2006.11 香港科技大學哲學博士(大氣環境科學

2006.11 – 2015.11 香港科技大學博士后、副研究員、研究助理教授、霍英東研究院大氣研究中心經理

2015.12 – 華南理工大學教授

2017.3入選“大氣污染成因與控制技術研究”重點專項視頻評審專家

招生專業

招生專業:083000環境科學與工程(學術型博士、學術型碩士)、 085229環境工程(專業學位碩士);截止到2018年,袁自冰教授團隊擁有博士研究生5名,碩士研究生8名(包含已經畢業碩士研究生一名),畢業設計本科生多名

主持項目

1.國家自然科學基金委“中國大氣復合污染的成因、健康影響和應對機制”聯合重大研究計劃重點支持項目“氣候變化背景下光化學活躍區大氣氧化性演變對近地面臭氧污染的影響研究”(91644221),250萬元(直接費用),2017.1-2020.12

2.國家重點研發計劃“大氣污染成因與控制技術研究”試點專項項目課題“大氣反應性有機化合物來源量化與校驗”(2016YFC0202201),730萬元,2016.7-2020.6

3.上海市科委科研計劃重點項目課題“上海市臭氧非線性變化控制機制研究”(16DZ204605),70萬元,2016.7-2018.6

4.華南理工大學中央高校基本科研業務費重點項目“珠三角二次有機氣溶膠估算方法研究”,20萬元,2015.7-2017.6

研究方向

研究方向概述:

近年來,由于一系列減排措施的推行,我國主要城市群大氣細顆粒物(PM2.5)污染得到一定程度的改善。然而,臭氧污染日益嚴重,引起政府和公眾的廣泛關注。國外的相關經驗表明,臭氧治理比PM2.5要困難的多,需要時間也長的多。我國現階段普遍采取的以PM2.5為導向的控制策略不能滿足臭氧控制的需求,在PM2.5達標后,我國主要城市群的大氣污染控制勢必轉移到以臭氧為防控重點上來。以長三角、珠三角等典型光化學活躍區近地面臭氧污染為研究核心,在反應性有機化合物排放特征、臭氧非線性變化控制機制以及氣候變化背景下大氣氧化性演變對近地面臭氧污染影響等方向開展深入研究,具體為:

1. 大氣反應性有機物來源量化與校驗:

反應性有機物在大氣化學過程和臭氧生成中起至關重要的作用,但其排放特征和化學轉化尚未得到充分研究。針對當前反應性有機物來源研究的兩個薄弱環節:活性組分測量和化學轉化過程校正,借助源排放測量、排放模型和文獻調研等手段,完善長三角和珠三角地區反應性有機物重要排放源化學成分譜,特別是補充現有反應性有機物源譜中缺失的支鏈烯烴、反應性醛類等關鍵活性組分,構建本地化的反應性有機物排放源數據庫;以2016年為基準年,構建中國東部地區高時空分辨率的反應性有機物排放源清單;針對反應性有機物重要排放源,量化表征大氣中反應性有機物從源到受體點的化學轉化過程,建立基于地面觀測、模型反演和衛星遙感的反應性組分來源校驗方法;并預估長三角和珠三角地區反應性有機物未來5~10年的排放趨勢。

2. 光化學活躍區臭氧非線性變化控制機制研究:

通過結合基于觀測模型、三維空氣質量模型和衛星遙感等三種技術手段,定量識別不同氣象條件下本地生成及區域傳輸對長三角和珠三角不同地區臭氧的相對貢獻,闡明不同地區臭氧及其前體物的非線性關系及其時空變化特征,揭示不同氣象條件下VOC敏感、NOx敏感及過渡區的空間分布;利用長期衛星遙感資料闡明長三角和珠三角地區評判VOC敏感、NOx敏感及過渡區的FNR標準,識別兩區域臭氧控制機制的長期變化趨勢,探索臭氧生成的敏感區域劃分隨NOx及揮發性有機物削減的變化規律,為遏制臭氧污染事件發生的頻率和強度以及制定中長期臭氧達標規劃提供科學依據。

3. 氣候變化背景下大氣氧化性演變對近地面臭氧污染影響研究:

臭氧防控通常需要數十年的時間,在這一時間尺度上氣候變化對臭氧污染的影響不可忽視。根據長三角和珠三角多站點長期監測結果,建立描述臭氧、NOx及環境溫度關系的概念模型,識別溫度對不同區域臭氧生成效率的影響;將溫度因素納入排放源清單動態體系,在不同環境溫度下對部分揮發性揮發性有機物排放源譜進行現場采樣與分析,闡明溫度對揮發性VOCs排放特征的影響;在本地化的三維空氣質量模型中應用納入溫度因素的動態排放源清單并對環境溫度進行擾動,揭示兩區域的臭氧氣候補償效應,建立溫度與臭氧前體物響應關系之間的函數關系,為不同氣候變化背景下兩區域制定臭氧控制策略提供科學依據。

主要貢獻

國際學術論文

1. Huang, Z.J., Hu, Y.T., Zheng, J.Y.*, Yuan, Z.B., Russell, A.G.*, Ou, J.M. and Zhong, Z.M. A new combined stepwisebased high-order decoupled direct and reduced-form method to improve uncertainty analysis in PM2.5 simulations, Environmental Science and Technology, 2017, 51, 3852-3859.

2. Zhong, Z.M., Sha, Q.E., Zheng, J.Y.*, Yuan, Z.B., Gao, Z.J., Ou, J.M., Zheng, Z.Y., Li, C. and Huang, Z.J. sectorbased 揮發性有機物 emission factors and source profiles for the surface coating industry in the Pearl River Delta region of China, Science of the 道達爾公司 Environment, 2017, 583, 19-28.

3. Yin, X.H., Huang, Z.J., Zheng, J.Y.*, Yuan, Z.B., Zhu, 微博電子競技俱樂部, Huang, X.B. and Chen, D.H. Source contributions to PM2.5 in Guangdong province, China by numerical modeling: results and implications, Atmospheric Research, 2017, 186, 63-71.

4. Ou, J.M., Yuan, Z.B.*, Zheng, J.Y.*, Huang, Z.J., Shao, M., Li, Z.K., Huang, X.B., Guo, H. and Louie, P.K.K. Ambient 臭氧 control in a photochemically active region: short-term despiking or long-term attainment?, Environmental Science and Technology, 2016, 50, 5720-5728.

5. Xue, J., Yuan, Z.B., Griffith, M., Yu, X., Lau, 安德烈·基里連科H. and Yu, J.Z.* Sulfate formation enhanced by a cocktail of High NOx, 二氧化硫, particulate matter, and droplet pH during haze-fog events in megacities in China: an observation-based modeling investigation, Environmental Science and Technology, 2016, 50, 7325-7334.

6. Li, C., Yuan, Z.B., Ou, J.M., Fan, X.L., Ye, S.Q., Xiao, T., Shi, Y.Q., Huang, Z.J., Ng, S.K.W., Zhong, Z.M. and Zheng, J.Y.* An AIS-based high-resolution ship emission inventory and its uncertainty in the Pearl River Delta region, China, Science of the Total Environment, 2016, 573, 1-10.

7. Lin, C.Q., Li, C.C.*, Lau, 安德烈·基里連科H., Yuan, Z.B., Lu, X.C., Tse, KT Rolster, Fung, J.C.H., Li, Y., Yao, T. and Su, L. Assessment of satellite-based aerosol optical depth using continuous lidar observation, Atmospheric Environment, 2016, 140, 273-282.

8. Yin, S.S., Zheng, J.Y.*, Lu, Q., Yuan, Z.B., Huang, Z.J., Zhong, L.J. and Lin, H. A refined 2010-based VOC emission inventory and its improvement on modeling regional 臭氧 in the Pearl River Delta region, China, Science of the Total Environment, 2015, 154, 426-438.

9. Li, Z.Y., Yuan, Z.B.*, Lau, A.K.H. and Louie, P.K.K. Characterization and source apportionment of health risks from ambient PM10 in Hong Kong over 2000-2011, Atmospheric Environment, 2015, 122, 892-899.

10. Su, L., Yuan, Z.B.*, Fung, J.C.H. and Lau, A.K.H. A comparison of HYSPLIT backward trajectories generated from two GDAS datasets, Science of the Total Environment, 2015, 506-507, 527-537.

11. Lin, C.Q., Li, Y.*, Yuan, Z.B., Lau, 安德烈·基里連科H., Li, C.C. and Fung, J.C.H. Using satellite remote sensing data to estimate the high-resolution distribution of ground-level PM2.5, Remote Sensing of Environment, 2015, 56, 117-128.

12. Huang, Z.J., Wang, S.S., Zheng, J.Y.*, Yuan, Z.B., Ye, S.Q. and Kang, D.W. Modeling inorganic nitrogen deposition in Guangdong province, China, Atmospheric Environment, 2015, 109, 147-160.

13. Yin, S.S., Zheng, J.Y.*, Lu, Q., Yuan, Z.B., Huang, Z.J., Zhong, L.J. and Lin, H. A refined 2010-based VOC emission inventory and its improvement on modeling regional 臭氧 in the Pearl River Delta region, China, Science of the Total Environment, 2015, 154, 426-438.

14. Xue, J., Yuan, Z.B.*, Yu, J.Z. and Lau, A.K.H. An observation-based model for secondary inorganic aerosols, Aerosol and Air Quality Research, 2014, 14, 862-878.

15. Xue, J., Yuan, Z.B., Lau, 安德烈·基里連科H. and Yu, J.Z.* Insights into factors affecting nitrate in PM2.5 in a polluted high NOx environment through hourly observations and size distribution measurements, Journal of Geophysical Research– Atmospheres, 2014, 119, 4888-4902.

16. Yu, X., Yuan, Z.B., Fung, J.C.H., Xue, J., Li, Y., Zheng, J.Y. and Lau, A.K.H.* 臭氧 changes in response to the heavy-duty diesel truck control in the Pearl River delta, Atmospheric Environment, 2014, 88, 269-274.

17. Yuan, Z.B., Yadav, V., Turner, J.R., Louie, P.K.K. and Lau, A.K.H.* Long-term trends of ambient particulate matter emission source contributions and the accountability of control strategies in Hong Kong over 1998-2008, Atmospheric Environment, 2013, 76, 21-31.

18. Yuan, Z.B., Zhong, L.J., Lau, 安德烈·基里連科H.*, Yu, J.Z. and Louie, P.K.K. Volatile organic compounds in the Pearl River Delta: Identification of source regions and recommendation for emission-oriented monitoring strategies, Atmospheric Environment, 2013, 76, 162-172.

19. Zhong, L.J., Louie, P.K.K.*, Zheng, J.Y., Wai, K.M., Ho, J.W.K., Yuan, Z.B., Lau, A.K.H., Yue, D.L. and Zhou, Y. The Pearl River Delta regional air quality monitoring network– regional collaborative efforts on joint air quality 管理學, Aerosol and Air Quality Research, 2013, 13, 1582-1597.

20. Deng, X.J.*, Wu, D., Yu, J.Z., Lau, 安德烈·基里連科H., Li, F., Tan, H.B., Yuan, Z.B., Ng, 威廉與瑪麗學院, Deng, T., Wu, C. and Zhou, X.J. Characterization of secondary aerosol and its extinction effects on visibility over the Pearl River Delta Region, China, Journal of Air and Waste 管理學 Association, 2013, 63, 1012-1021.

21. Zhong, L.J., Louie, P.K.K.*, Zheng, J.Y., Yuan, Z.B., Yue, D.L., Ho, J.W.K. and Lau, A.K.H. Science-policy Interplay娛樂: Air quality management in the Pearl River Delta and Hong Kong, Atmospheric Environment, 2013, 76, 3-10.

22. Lu, Q., Zheng, J.Y.*, Ye, 世界樹迷宮, Shen, X.L., Yuan, Z.B. and Yin, S.S. Emission trends and source characteristics of 二氧化硫, NOx, PM10 and 揮發性有機物 in the Pearl River Delta region from 2000 to 2009, Atmospheric Environment, 2013, 76, 11-20.

23. Louie, P.K.K.*, Ho, J.W.K., Tsang, R.C.W., Blake, D.R., Lau, 安德烈·基里連科H., Yu, J.Z., Yuan, Z.B., Wang, X.M., Shao, M. and Zhong, L.J. VOCs and OVOCs distribution and control policy implications in Pearl River Delta region, China, Atmospheric Environment, 2013, 76, 125-135.

24. Li, Y.C., Yu, J.Z.*, Ho, S.S.H., Schauer, 約翰·約翰遜, Yuan, Z.B., Lau, A.K.H. and Louie, P.K.K. Chemical characteristics and source apportionment of fine particulate organic carbon in Hong Kong during high particulate matter episodes in winter 2003, Atmospheric Research, 2013, 120, 88-98.

25. Li, Y.C., Yu, J.Z.*, Ho, S.S.H., Yuan, Z.B., Lau, 安德烈·基里連科H. and Huang, X.F. Chemical characteristics of PMand organic aerosol source analysis during cold front episodes in Hong Kong, China, Atmospheric Research, 2012, 118, 41-51.

26. Zheng, J.Y.*, He, M., Shen, X.L., Yin, S.S. and Yuan, Z.B. High resolution of 黑色 carbon and organic carbon emissions in the Pearl River Delta region, China, Science of the Total Environment, 2012, 438, 189-200.

27. Lau, A.K.H., Yuan, Z.B.*, Yu, J.Z. and Louie, P.K.K. Source apportionment of ambient volatile organic compounds in Hong Kong, Science of the Total Environment, 2010, 408, 4138-4149.

28. Yuan, Z.B., Lau, 安德烈·基里連科H.*, Shao,M., Louie, P.K.K., Liu, S.C. and Zhu, T. Source analysis of volatile organic compounds by positive matrix factorization in urban and rural environments in Beijing, Journal of Geophysical Research, 2009, 114,doi:10.1029/2008JD011190.

29. Huang, X.F., Yu, J.Z.*, Yuan, Z.B., Lau, A.K.H. and Louie, P.K.K. Source analysis of high particulate matter days in Hong Kong, Atmospheric Environment, 2009, 43, 1196-1203.

30. Yuan, Z.B., Lau, A.K.H.*, Zhang, H.Y., Yu, J.Z., Louie, P.K.K. and Fung, J.C.H. Identification and spatiotemporal variation of dominant PMsources over Hong Kong, Atmospheric Environment, 2006, 40, 1803-1815.

31. Yuan, Z.B., Yu, J.Z.*, Lau, A.K.H., Louie, P.K.K. and Fung, J.C.H. Application of positive matrix factorization in estimating aerosol secondary organic carbon in Hong Kong and its relationship with secondary sulfate, Atmospheric 化學 and Physics, 2006, 6, 25-34.

32. Huang, X.F., Yu, J.Z.*, He, L.Y. and Yuan, Z.B. Water-soluble organic carbon and oxalate in aerosols at a coastal urban site in China: Size distribution characteristics, sources and formation mechanisms, Journal of Geophysical Research, 2006, 111,doi:10.1029/2006JD007408.

33. Lo, JC·弗勞爾斯公司, Lau, 安德烈·基里連科H.*, Yuan, Z.B., Chen, F. and Fung, J.C.H. A physical modeling approach for identification of source regions of air pollutants, Atmospheric Chemistry and Physics Discussions, 2006, 6, 6467-6496.

34. Li, C.C., Mao, J.T.*, Lau, A.K.H., Yuan, Z.B., Wang, M.H. and Liu, X.Y. Application of MODIS satellite products to the air pollution research in Beijing, Science in China Series D– Earch Sciences, 2005, 48, Suppl. 2, 209-219.

35. Li, C.C., Mao, J.T.*, Lau, A.K.H., Chen, J.C., Yuan, Z.B., Liu, X.Y., Zhu, A.H. and Liu, G.Q. Characteristics of distribution and seasonal variation of aerosol optical depth in eastern China with MODIS products, Chinese Science Bulletin, 2003, 48, 2488-2495.

36. Fung, J.C.H.*, Lau, A.K.H., Lam, J.S.L. and Yuan, Z.B. Observational and modeling analysis of a severe air pollution episode in western Hong Kong. Journal of Geophysical Research, 2003, 110,doi: 10.1029/2004JD005105.

參考資料 >

華南理工大學環境與能源學院.華南理工大學環境與能源學院.2018-07-27

國家重點研發計劃“大氣污染成因與控制技術研究”重點專項2017年度指南申報項目視頻評審專家名單公告.國家重點研發計劃“大氣污染成因與控制技術研究”重點專項2017年度指南申報項目視頻評審專家名單公告.2018-07-27

重點研發計劃.重點研發計劃三個重點專項視頻答辯評審專家名單.2018-07-29

Insights into factors affecting nitrate in PM2.5 in a polluted high NOx environment through hourly observations and size distribution measurements.JGR.2018-07-29

The Pearl River Delta regional air quality monitoring network– regional collaborative efforts on joint air quality management.AAQR.2018-07-29

Characterization of secondary aerosol and its extinction effects on visibility over the Pearl River Delta Region, China.JAWMA.2018-07-29

Characteristics of distribution and seasonal variation of aerosol optical depth in eastern China with MODIS products.CSB.2018-07-29

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